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Ion trap cavity quantum electrodynamics

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ION TRAP CAVITY QUANTUM ELECTRODYNAMICS CHUAH BOON LENG B.Sc. (Hons.), NUS A THESIS SUBMITTED FOR THE DEGREE OF DOCTOR OF PHILOSOPHY IN PHYSICS DEPARTMENT OF PHYSICS NATIONAL UNIVERSITY OF SINGAPORE 2013 Declaration of Authorship I hereby declare that this thesis is my original work and it has been written by me in its entirety. I have duly acknowledged all the sources of information which have been used in the thesis. This thesis has also not been submitted for any degree in any university previously. Signed: Date: 4th December 2013 i Acknowledgements The completion of my project would be impossible without the support from my family. I have to thank my parents for their unconditional loves and supports, which give me peace of mind and keep me going all the way. I also have to thank my sister, who has been taking good care of my parents all these years. I am very grateful to my wife, Mei Fei; my life would definitely be a mess without her spiritual supports and guidances. Of course I have to thank my supervisor, Murray, who welcomed me in his group and taught me everything from aligning optics to writing manuscripts. A special thank to Meng Khoon, for giving me his invaluable advices all these years. If I were to build all the experimental setup by myself, the project would never come to a completion. For this, I owe 50% of my achievements to Nick, who has been my project mate all along. A big thank you to Markus, for his significant contribution to my first publication and the useful discussions we had when I was struggling hard with writing manuscripts or solving theoretical problems. Equally important are Kyle and Radu, their constructive comments and advices on various aspects are deeply appreciated. Thanks to Joven and Andrew, for providing technical supports from machining to technical drawing. I am also very thankful for the joy and laughter brought by Arpan, which comforted me and others even when things went really wrong in the lab. To my other friends, thanks for supporting me during the bad times and celebrating with me during the good. It has been a great experience for me to work on this project. Although the journey has never been easy, in the end I realize that every obstacle I came across was actually a stepping stone towards success. Therefore, I am proud and grateful for being part of my team: Microtrap group. ii Contents Declaration of Authorship i Acknowledgements ii Abstract vii List of Publications viii List of Tables ix List of Figures x Abbreviations xii Introduction Theoretical Considerations 2.1 Linear Paul Trap . . . . . . . . . . . . . . . . . . . . . . . 2.2 Doppler Cooling . . . . . . . . . . . . . . . . . . . . . . . . 2.3 Coherent State Manipulation of Trapped Ions . . . . . . . 2.3.1 Overview . . . . . . . . . . . . . . . . . . . . . . . 2.3.2 Raman Transitions . . . . . . . . . . . . . . . . . . 2.3.2.1 Phase Fluctuations . . . . . . . . . . . . . 2.3.2.2 Motional Coupling . . . . . . . . . . . . . 2.3.3 Raman Sideband Cooling . . . . . . . . . . . . . . 2.4 Cavity QED: A Brief Theoretical Overview . . . . . . . . . 2.5 Thermal Effect on Ion-cavity Coupling . . . . . . . . . . . 2.6 Cavity Cooling in the Presence of Recoil Heating and Cavity Birefringence . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 4 10 10 11 14 15 17 18 24 . 27 Apparatus 30 3.1 The Ion Trap . . . . . . . . . . . . . . . . . . . . . . . . . . 30 3.2 The Experimental Cavity . . . . . . . . . . . . . . . . . . . . 34 iii Contents 3.3 3.4 3.5 3.6 3.7 3.2.1 The Cavity Design . . . . . . . . . . . . . . . . . . 3.2.2 Detection of the Cavity Emission . . . . . . . . . . The Imaging System . . . . . . . . . . . . . . . . . . . . . The General Considerations of the Laser System . . . . . . 3.4.1 Overview . . . . . . . . . . . . . . . . . . . . . . . 3.4.2 The Transfer-Cavity-Lock . . . . . . . . . . . . . . 3.4.3 The Self-heterodyne Locking System . . . . . . . . 3.4.3.1 Theory . . . . . . . . . . . . . . . . . . . 3.4.3.2 Implementation . . . . . . . . . . . . . . . The Doppler Cooling Lasers . . . . . . . . . . . . . . . . . 3.5.1 The 493 nm Laser System . . . . . . . . . . . . . . 3.5.1.1 The 986 nm laser . . . . . . . . . . . . . . 3.5.1.2 The doubling cavity . . . . . . . . . . . . 3.5.1.3 The EOM and AOM setup . . . . . . . . 3.5.2 The 650 nm Laser System . . . . . . . . . . . . . . 3.5.2.1 The laser frequency stabilization . . . . . 3.5.2.2 The repumping system for 137 Ba+ . . . . . The Raman Lasers . . . . . . . . . . . . . . . . . . . . . . 3.6.1 The Red Cavity . . . . . . . . . . . . . . . . . . . . 3.6.2 The 493 nm Raman Laser . . . . . . . . . . . . . . 3.6.3 The 650 nm Laser . . . . . . . . . . . . . . . . . . . The Synchronization Between the Experimental Cavity and the Cavity Probing Laser . . . . . . . . . . . . . . . . . . . 3.7.1 The Blue Cavity . . . . . . . . . . . . . . . . . . . 3.7.2 The Compensation for the Fast Jitter in the Experimental Cavity . . . . . . . . . . . . . . . . . Experimental Methods 4.1 Ion Loading . . . . . . . . . . . . . . . . . . . . . . . . . 4.1.1 Barium Oven . . . . . . . . . . . . . . . . . . . . 4.1.2 Photo-ionization . . . . . . . . . . . . . . . . . . 4.2 Temperature Measurement of 138 Ba+ . . . . . . . . . . . 4.3 Two-color Raman Cooling of 138 Ba+ . . . . . . . . . . . 4.4 General Methods in Cavity QED Experiments . . . . . . 4.4.1 Cavity Linewidth Measurements . . . . . . . . . . 4.4.2 Alignment of the Cavity Field to a Single Ion . . 4.4.3 Ion-Cavity Emission Profiles . . . . . . . . . . . . 4.4.3.1 Birefringence induced phase retardation 4.4.4 The Single Atom Cooperativity . . . . . . . . . . 4.5 The Cavity-Enhanced Single Ion Spectroscopy . . . . . . 4.5.1 Overview . . . . . . . . . . . . . . . . . . . . . . iv . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 34 35 36 38 38 40 43 43 44 47 47 48 49 50 50 50 52 54 54 56 56 . 58 . 59 . 61 . . . . . . . . . . . . . 63 64 64 65 66 70 75 75 76 77 79 81 83 83 Contents 4.5.2 4.5.3 4.5.4 Methods . . . . . . . . . . . . . . . . . . . . . . . . . 84 Measurements . . . . . . . . . . . . . . . . . . . . . . 86 Results . . . . . . . . . . . . . . . . . . . . . . . . . . 87 State Detection Using Coherent Raman Repumping and Two-color Raman Transfer 89 5.1 The Concepts . . . . . . . . . . . . . . . . . . . . . . . . . . 90 5.2 Experimental Setup . . . . . . . . . . . . . . . . . . . . . . . 93 5.3 Experiments . . . . . . . . . . . . . . . . . . . . . . . . . . . 93 5.3.1 State Preparation . . . . . . . . . . . . . . . . . . . . 93 5.3.2 Results . . . . . . . . . . . . . . . . . . . . . . . . . . 95 5.3.3 The Limiting Factors . . . . . . . . . . . . . . . . . . 95 5.4 Two-color Raman Transfer . . . . . . . . . . . . . . . . . . . 99 5.5 Concluding Remarks . . . . . . . . . . . . . . . . . . . . . . 101 Detection of Ion Micromotion in a Linear a High Finesse Cavity 6.1 Introduction . . . . . . . . . . . . . . . . . 6.2 The Model . . . . . . . . . . . . . . . . . . 6.3 The Experiment . . . . . . . . . . . . . . . 6.4 Results . . . . . . . . . . . . . . . . . . . . 6.5 Limiting Factors . . . . . . . . . . . . . . 6.6 Concluding Remarks . . . . . . . . . . . . Sub-Doppler Cavity Cooling Regime 7.1 Cavity Cooling . . . . . . . . 7.2 Setup . . . . . . . . . . . . . . 7.3 Experiments . . . . . . . . . . 7.4 Concluding Remarks . . . . . Paul Trap with 102 . . . . . . . . . . 102 . . . . . . . . . . 104 . . . . . . . . . . 108 . . . . . . . . . . 111 . . . . . . . . . . 114 . . . . . . . . . . 115 Beyond The Lamb-Dicke 116 . . . . . . . . . . . . . . . . . 117 . . . . . . . . . . . . . . . . . 118 . . . . . . . . . . . . . . . . . 119 . . . . . . . . . . . . . . . . . 122 Photon Statistics of the Ion-Cavity Emission 8.1 Model . . . . . . . . . . . . . . . . . . . . . . 8.2 Experiments . . . . . . . . . . . . . . . . . . . 8.3 Results . . . . . . . . . . . . . . . . . . . . . . 8.4 Concluding Remarks . . . . . . . . . . . . . . Conclusions . . . . . . . . . . . . . . . . . . . . . . . . . . . . 123 . 123 . 127 . 128 . 130 132 A Barium Atomic and Ionic Data 135 A.1 Basic Atomic Data . . . . . . . . . . . . . . . . . . . . . . . 135 v Contents A.2 Ionic Transition Data . . . . . . . . . . . . . . . . . . . . . . 136 B The Probability Distribution of a Leaky State 143 Bibliography 146 vi Abstract A trapped ion-cavity system is a potential candidate in quantum information processing (QIP) applications as it provides an efficient interface between ions (quantum memory) and photons (information carrier). In addition, a cavity also provides other useful functions for a trapped ion system such as ion cooling. This thesis explores various functionalities of a trapped ion-cavity system that highlight its potential as a practical tool for QIP applications. In this thesis, experiments are performed on a singly charged barium ion trapped within a high finesse cavity. The experiments make use of a vacuum stimulated Raman transition, which involves an exchange of one photon between the driving laser operating at 493 nm and the intra-cavity field with a resonance at the same wavelength. Depending on the experimental goal, the system can be manipulated to induce mechanical effects on the trapped ion or alter the properties of the cavity output. Using these approaches, the following experimental results are reported: efficient 3-D micromotion compensation despite optical access limitations imposed by the cavity mirrors, first demonstration of sub-Doppler cavity sideband cooling of trapped ions, and first proposal of ion temperature probing using a high finesse cavity. Additionally, a number of useful techniques such as cavity enhanced single ion spectroscopy and state detection using Raman repumping lasers were developed over the course of the experiments. vii List of Publications The following is a list of publications I have coauthored during my Ph.D. studies. 1. Boon Leng Chuah, Nicholas C. Lewty, and Murray D. Barrett. State detection using coherent raman repumping and two-color raman transfers. Physical Review A, 84:013411, Jul 2011. 2. Nicholas C. Lewty, Boon Leng Chuah, Radu Cazan, B. K. Sahoo, and M. D. Barrett. Spectroscopy on a single trapped 137 Ba+ ion for nuclear magnetic octupole moment determination. Optics Express, 20(19):21379–21384, Sep 2012. 3. Boon Leng Chuah, Nicholas C. Lewty, Radu Cazan, and Murray D. Barrett. Sub-doppler cavity cooling beyond the lamb-dicke regime. Physical Review A, 87:043420, Apr 2013. 4. Boon Leng Chuah, Nicholas C. Lewty, Radu Cazan, and Murray D. Barrett. Detection of ion micromotion in a linear paul trap with a high finesse cavity. Optics Express, 21(9):10632–10641, May 2013. 5. Nicholas C. Lewty, Boon Leng Chuah, Radu Cazan, B. K. Sahoo, and M. D. Barrett. Experimental determination of the nuclear magnetic octupole moment of 137 012518, Jul 2013. viii Ba+ ion. Physical Review A, 88: List of Tables 3.1 3.2 Properties of trap A and B . . . . . . . . . . . . . . . . . . . 32 The AOM frequencies of 650 nm repumper . . . . . . . . . . 53 A.1 A.2 A.3 A.4 . 135 . 136 . 136 Isotopes of barium . . . . . . . . . . . . . . . . . . . . . . Isotopes shift @ 493 nm and 455 nm . . . . . . . . . . . . . Isotopes shift @ 650 nm, 614 nm, and 585 nm . . . . . . . . Dipole matrix elements for transition J = 1/2 → J = 1/2 of isotopes with In = . . . . . . . . . . . . . . . . . . . . A.5 Dipole matrix elements for transition J = 3/2 → J = 1/2 of isotopes with In = . . . . . . . . . . . . . . . . . . . . A.6 135 Ba+ or 137 Ba+ relative hyperfine transition strength for P1/2 → S1/2 . . . . . . . . . . . . . . . . . . . . . . . . . . A.7 135 Ba+ or 137 Ba+ relative hyperfine transition strength for P1/2 → D3/2 . . . . . . . . . . . . . . . . . . . . . . . . . . A.8 135 Ba+ or 137 Ba+ hyperfine dipole matrix elements for transition S1/2 | F = → P1/2 | F = . . . . . . . . . . . A.9 135 Ba+ or 137 Ba+ hyperfine dipole matrix elements for transition S1/2 | F = → P1/2 | F = . . . . . . . . . . . A.10 135 Ba+ or 137 Ba+ hyperfine dipole matrix elements for transition S1/2 | F = → P1/2 | F = . . . . . . . . . . . A.11 135 Ba+ or 137 Ba+ hyperfine dipole matrix elements for transition S1/2 | F = → P1/2 | F = . . . . . . . . . . . A.12 135 Ba+ or 137 Ba+ hyperfine dipole matrix elements for transition D3/2 | F = → P1/2 | F = . . . . . . . . . . . A.13 135 Ba+ or 137 Ba+ hyperfine dipole matrix elements for transition D3/2 | F = → P1/2 | F = . . . . . . . . . . . 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Physical Review A, 88: [...]... generations of entanglement between two trapped ions [11], creations of a quantum byte by deterministically entangling eight calcium ions [12], quantum teleportations [13] and implementations of Grovers search algorithm [14] have all been realized experimentally with trapped ions Moreover, recent demonstrations of entanglements between trapped ions and photons [15], and between distant trapped ions [16,... ideal system for such an interface is based on an ion trapped within a high finesse cavity [20–22] The cavity enhances the interaction between the ion and a single photon, and enables efficient collection of the ion emissions Proposed applications of trapped ion- cavity systems in QIP include quantum repeaters [23, 24], entanglement of distant ions [25–27] and quantum logic gates [28–31] To date, remarkable... sources [21, 32], single ion lasers [33] and ion- photon entanglement [22] have all been demonstrated with trapped ion- cavity setups In addition to QIP applications, a cavity also provides other useful functions for a trapped ion system such as enhanced photon collection efficiency [34] and a means for cooling ions [35] As a progression in exploring the various functionalities of a cavity, this thesis presents... of an ion trap for confining singly charged barium ions is described Afterwards, the principle of ion trap Doppler cooling is presented in Section 2.2 In Section 2.3, a brief introduction of coherent population transfer is discussed Then a theoretical overview of cavity QED is presented in Section 2.4, which is followed by two sections discussing the thermal effects on ion- cavity coupling and cavity. .. the phases determined by the initial conditions of the ion position and velocity The solutions of Equation 2.7 and Equation 2.8 comprise motions in two timescales, corresponding to the secular motion and the micromotion The secular motion is the harmonic oscillation of the ion with the amplitude Ax,y,z and the frequency ωx,y,z , while the micromotion is motion driven by the RF field and is scaled by... Photo-ionization scheme Temperature measurement procedure Raman spectra of vibrational modes Raman cooling scheme Cavity birefringence Cavity output vs Attocube motion Ion- cavity emission profiles Birefringence induced phase retardation Single atom cooperativity Cavity- enhanced single ion spectroscopy setup Cavity- enhanced... Paul trap Stable zone of an ion trap The Λ-type Raman Transition Ion- cavity Raman coupling The setup for ion- cavity coupling 6 7 11 20 23 3.1 3.2 3.3 3.4 3.5 3.6 3.7 3.8 3.9 3.10 3.11 3.12 3.13 The trap picture A schematic diagram of trap B Home-build transformer Experimental cavity Trap. .. used such as ion trapping using radio frequency (RF) traps, Doppler cooling of trapped ions and atomic state manipulation Then the theory for an ideal two-level atom in an optical cavity is presented The description is later extended to include the realistic considerations, such as cavity and excited state dissipations, and the effects due to external driving lasers Before 2 Chapter 1 Introduction the chapter... used to further reduce the ion temperature As seen in the previous section, a Λ-type Raman transition could be motional sensitive depending on the laser configuration With an appropriate setting, the Raman transition can transfer the ion from a higher vibration quantum to a lower one and reduce the ion temperature 17 Chapter 2 Theoretical Considerations Here, a brief description of the cooling process... 6.4 Micromotion detection by cavity: setup Relevant transitions and level structure Micromotion sidebades at different stages Cavity profile when fully compensated 105 109 112 113 7.1 7.2 7.3 Cavity cooling setup 118 Relevant transitions 119 Cavity cooling data 120 8.1 8.2 Cavity emission profile . enhances the interaction between the ion and a single photon, and enables efficient collection of the ion emissions. Proposed applications of trapped ion- cavity systems in QIP include quantum repeaters. demonstrated with trapped ion- cavity setups. In addition to QIP applications, a cavity also provides other useful functions for a trapped ion system such as enhanced photon collection efficiency [34]. generations of entanglement between two trapped ions [11], creations of a quantum byte by deterministically entangling eight calcium ions [12], quantum teleportations [13] and implementations of

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