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STAPPA
State and Territorial Air Pollution
Program Administrators
ALAPCO
Association of Local Air
Pollution Control Ofcials
March 2006
Controlling
Fine ParticulateMatter
Under theCleanAirAct:
A Menuof Options
STAPPA
State and Territorial Air Pollution
Program Administrators
ALAPCO
Association of Local Air
Pollution Control Offi cials
March 2006
Controlling
Fine ParticulateMatter
Under theCleanAirAct:
A Menuof Options
Acknowledgements i
Acknowledgements
On behalf ofthe State and Territorial Air Pollution
Program Administrators (STAPPA) and the Association
of Local Air Pollution Control Offi cials (ALAPCO),
we are pleased to provide ControllingFineParticulate
Matter UndertheCleanAirAct:AMenuof Options. Our
associations developed this document to assist states and
localities in determining the most effective ways to control
emissions of fi ne particles (PM
2.5
) and PM
2.5
precursors
from sources in their areas. We hope that states and
localities fi nd this document useful as they prepare
their State Implementation Plans (SIPs) for attaining or
maintaining the PM
2.5
standard.
STAPPA and ALAPCO express gratitude to M.J Bradley
& Associates, Inc. for its assistance in drafting this
document, in particular, Ann Berwick, Michael Bradley,
Tom Curry, Will Durbin, Dana Lowell and Chris Van
Atten. We thank Brock Nicholson (North Carolina) and
Lynne Liddington (Knox County, Tennessee), co-chairs
of the associations’ Criteria Pollutants Committee, under
whose guidance this document was prepared. We also
appreciate the efforts ofthe STAPPA and ALAPCO PM
2.5
Menu ofOptions Review Workgroup, who helped shape
the options presented in this document. We thank Bill
Becker, Executive Director of STAPPA and ALAPCO, and
Amy Royden-Bloom, Senior Staff Associate of STAPPA
and ALAPCO, who oversaw the project. Finally, we
express our gratitude to EPA for providing the funding for
this project.
Once again, we believe that ControllingFineParticulate
Matter UndertheCleanAirAct:AMenuofOptions
will serve as a useful and important resource for states
and localities as they develop approaches to regulate
emissions of PM
2.5
and PM
2.5
precursors and thank all who
contributed to its development.
Eddie Terrill John Paul
STAPPA President ALAPCO President
Contents iii
Contents
Introduction 1
Chapter 1. The Highlights 5
Chapter 2. Effects ofParticulateMatter on Human Health and the Environment 16
Chapter 3. FineParticulateMatter and Precursor Emissions 22
Chapter 4. TheCleanAir Act 32
Chapter 5. Boiler Technologies 42
Chapter 6. Industrial and Commercial Boilers 60
Chapter 7. Electric Generating Units 86
Chapter 8. Pulp and Paper 108
Chapter 9. Cement Manufacturing 120
Chapter 10. Iron and Steel 136
Chapter 11. Petroleum Refi neries 158
iv ControllingFineParticulateMatterUndertheCleanAirAct:AMenuof Options
Chapter 12. Diesel Engine Technologies 172
Chapter 13. Diesel Trucks and Buses 188
Chapter 14. Nonroad Equipment 202
Chapter 15. Light-Duty Cars and Trucks 216
Chapter 16. Airports 228
Chapter 17. Marine Ports 238
Chapter 18. Residential Fuel Combustion and Electricity Use 252
Chapter 19. Commercial Cooking 266
Chapter 20. Fugitive Dust 274
About STAPPA and ALAPCO v
The State and Territorial Air Pollution Program
Administrators (STAPPA) and the Association of Local
Air Pollution Control Offi cials (ALAPCO) are the two
national associations ofair quality offi cials in the states,
territories and major metropolitan areas throughout the
country. The members of STAPPA and ALAPCO have
primary responsibility for implementing our nation’s air
pollution control laws and regulations. The associations
serve to encourage the exchange of information and
experience among air pollution control offi cials; enhance
communication and cooperation among federal, state
About STAPPA and ALAPCO
and local regulatory agencies; and facilitate air pollution
control activities that will result in clean, healthful air
across the country. STAPPA and ALAPCO share joint
headquarters in Washington, DC.
For further information, contact STAPPA and ALAPCO at
444 North Capitol Street, NW, Suite 307, Washington, DC
20001 (telephone: 202-624-7864; fax: 202-624-7863; email
4cleanair@4cleanair.org) or visit our associations’ web site
at www.4cleanair.org.
Introduction 1
The State and Territorial Air Pollution Program
Administrators (STAPPA) and the Association of Local
Air Pollution Control Offi cials (ALAPCO) have prepared
Controlling FineParticulateMatterUndertheCleanAir
Act: AMenuofOptions (PM
2.5
Menuof Options) to assist
state and local air pollution control offi cials in evaluating
the options for reducing fi ne particulatematter (PM
2.5
) and
PM
2.5
-precursor emissions.
Areas throughout the eastern U.S. and California (and one
area in Montana) currently exceed EPA’s National Ambient
Air Quality Standards (NAAQS) for PM
2.5
, and states must
submit State Implementation Plans (SIPs) by April 2008
detailing their plans for achieving the national standards.
Meanwhile, the PM
2.5
NAAQS are once again undergoing
the periodic review that §109(d)(1) oftheCleanAir Act
requires take place at fi ve-year intervals. Underthe terms
of a consent decree, EPA is to issue fi nal standards by
September 27, 2006. The Agency proposed new standards
on January 17, 2006.
EPA estimates that meeting the current PM
2.5
standards
would avoid tens of thousands of premature deaths
annually and save hundreds of thousands of people from
signifi cant respiratory and cardiovascular disease. The
Agency further estimates that the monetized health
benefi ts of improvements in PM
2.5
air quality exceed the
costs by a substantial margin.
PM
2.5
is a complex pollutant with many sources
Introduction
contributing to the ambient air quality problem. As a
result, this PM
2.5
Menu ofOptions addresses a broad
array of emission source categories, ranging from
household furnaces to petroleum refi neries. The challenge
confronting air quality offi cials is tremendous, as
evidenced by the sheer number ofoptions that we identify
for improving air quality. But therein lie the opportunities,
as well.
Like STAPPA’s and ALAPCO’s previous document—
Controlling ParticulateMatterUndertheCleanAir
Act: AMenuof Options—this document compiles and
analyzes secondary information. It is intended to serve
as a general reference for a national audience, and it will
in no way substitute for a thorough analysis by state and
local agencies of local emissions sources and conditions,
using appropriate guidance from EPA and other available
information.
What To Regulate
The national focus of this report should not obscure an
absolutely central point: local choices about the sources
and pollutants to control will need to be informed by
highly local considerations. A particular source category
may account for a small share of national PM
2.5
emissions,
but it may nonetheless dominate the local inventory.
The chemistry and physics of PM
2.5
formation in the
atmosphere is incompletely understood. Some PM
2.5
is
2 ControllingFineParticulateMatterUndertheCleanAirAct:AMenuof Options
released directly to the atmosphere, and some forms from
emissions of sulfur dioxide (SO
2
) and nitrogen oxides
(NO
x
) (which are currently viewed as the most signifi cant
precursors and are the only ones addressed in this report).
Ammonia and volatile organic compounds (VOCs),
which are not included in this report, can also contribute
to ambient PM
2.5
. Direct PM
2.5
emissions may be largely
responsible for one area’s nonattainment, while SO
2
emissions may cause the problem elsewhere. The choice of
whether to focus on reducing direct PM
2.5
, SO
2
or NO
x
—or
all of them, or ammonia or VOCs—will depend on local
source contributions and atmospheric chemistry.
There are further challenges for SIP writers. In a perfect
world, control-effi ciency and cost-effectiveness data would
be at hand; however, it is not consistently available. Of
course, even when information of this sort can be found, it
may not be applicable to all sources.
And another source of uncertainty complicates the job.
As we discuss in Chapter 3, FineParticulateMatter and
Precursor Emissions, there are important distinctions
between fi lterable and condensable PM
2.5
. Further, some
methods used to measure PM emissions refl ect only the
fi lterable components and, to exacerbate the problem, the
fi lterable components vary depending on the test method
used. Although we discuss this issue in Chapter 3 in the
context ofthe national PM
2.5
inventory, the distinction
between fi lterables and condensables also raises regulatory
and permitting issues.
The Authority to Regulate
Having decided what sources and pollutants need to
be controlled in order to address PM
2.5
nonattainment,
regulators must then ascertain their authority to do so.
The CleanAir Act divides responsibility for various
types ofair pollution sources and air pollutants between
the states and localities on the one hand and the federal
government on the other. Generally, state and local
regulators share responsibility with EPA for regulating
so-called “criteria” pollutants from stationary and area
sources (see Chapter 4, TheCleanAir Act), with states and
localities assigned the lead role in addressing emissions
from these source categories.
States and localities are free under federal law to adopt
more stringent standards for stationary and area sources
than theCleanAir Act requires. However, some states
may be limited by state law or policy in whether they can
enact requirements that are more stringent than federal
standards. Here, we outline the possible approaches to
tightening federal standards that states and localities may
consider, and to developing standards where no federal
programs exist.
For states that have no latitude or little latitude beyond
what theCleanAir Act prescribes, the priority will be to
ensure strict compliance with the limits that the Act and
federal regulations impose on particulates and precursor
pollutants. In these states, the precise language ofthe
statutory limitation will inform the degree of regulatory
latitude. For example, regulators in at least some of these
states may not be able to set more stringent standards
for those sources that federal law or regulations actually
address, but in some of these states regulators may see
their way clear to setting standards for smaller sources
than those covered by federal requirements.
Moreover, there are no actual federal Reasonably Available
Control Technology (RACT) standards—EPA issues
only guidelines (and although the RACT standards are
intended to refl ect real-time advancements in technology,
many ofthe guidelines are seriously outdated). Since the
guidelines do not set actual limits, even state prohibitions
against enacting more stringent state standards may be
inapplicable.
States and localities that are not limited to the requirements
promulgated under federal law will want to look to the most
stringent standards that regulators in other jurisdictions
have imposed; we have identifi ed these throughout this
Menu of Options. State and local authority to impose
such limits derives from the federal requirement to attain
the NAAQS. Theoptions for imposing more stringent
requirements than current federal regulations include the
following:
Under the state or local version of federal regulatory
air pollution programs, or through permit
determinations, adopt the most stringent standards
that appear to be feasible, even if they are more
stringent than federal rules impose; or apply the
federal or stricter standards to sources that are smaller
than those covered by the federal requirements.
Craft state or local regulatory programs or permits
that impose on sources the most stringent standards
that appear to be feasible. For example, this might
include the imposition of Best Available Control
Tech nolog y (BACT)-level st anda rd s on existi ng
sources, even in the absence ofa modifi cation that
would trigger New Source Review (NSR).
Through regulations or permits, set limits on sulfur
levels in coal and oil for sources that burn these fuels.
For sources that are permitted to burn more than one
type of fuel, impose permit conditions that strictly
limit the extent to which they may burn the more
polluting fuel.
Consider the imposition of regulatory standards that
can be met by most, but not necessarily all, sources to
which the standard is applicable, with an opportunity
•
•
•
•
•
Introduction 3
for sources to demonstrate that the standards
are technically infeasible in light of particular
circumstances.
Adopt a state-level cap-and-trade program or
participate in a regional trading program for a
particular source category or group of source
categories.
The discussion above applies to stationary and area
sources, but not to mobile sources, as to which all states
other than California have less leeway to impose their own
standards. For new vehicles, states are limited to federal
standards or to the more stringent standards that California
has adopted. For existing onroad vehicles, all states can
impose their own standards; although for existing nonroad
vehicles, they once again have only the choice of federal or
California standards.
However, by no stretch ofthe imagination does this mean
that states should overlook the possibilities for mobile
source strategies as a way of tackling PM
2.5
nonattainment.
As we discuss in the chapters that follow, states have a
range of opportunities for addressing these sources.
Energy Effi ciency
The rising cost of fossil fuels has focused the nation’s
attention on the opportunities for reducing fuel
consumption, including energy effi ciency measures,
some of which are addressed in this report. For example,
Chapter 18, Residential Fuel Combustion and Electricity
Use, discusses several demand-side effi ciency measures.
However, other source categories surely present
opportunities for increased effi ciency that regulators
should not overlook.
On the supply side, energy effi ciency measures involve
increasing the effi ciency ofthe fuel combustion process or
of the way the fuel is utilized. At a conventional power
plant, two-thirds ofthe potential energy in the fuel burned
to produce electricity is inevitably lost to waste heat.
Meanwhile, facilities burn additional fuel to satisfy their
thermal needs (for hot water, space heating and the like).
Combined heat and power (CHP or cogeneration) facilities
located at or near a facility address this problem by
recovering the waste heat and putting it to productive use.
CHP systems can achieve overall effi ciencies of greater
than 80 percent (Elliott, 1999; EPA, 2000). In the late
1990s, 9 percent of this country’s electricity came from
cogeneration plants, although a number of other countries
garnered a much higher percentage: Denmark (40 percent),
Finland and the Netherlands (30 percent each), the Czech
Republic (18 percent), and Germany (15 percent) (Elliott,
1999).
A number ofthe industry sectors we profi le in this
•
report are candidates for cogeneration. The petroleum
refi ning and pulp and paper industries already employ
cogeneration to some degree, but the practice has room to
grow further in those industries and others, such as cement
manufacturing and iron and steel production (Elliott,
1999).
There are unquestionably disincentives to the development
of CHP in this country (e.g., high prices for excess power
that CHP projects sell to the grid, long tax depreciation
periods for CHP equipment), although increasing fuel
prices make cogeneration more attractive. Environmental
regulators can reverse some ofthe disincentives; for
example, by writing air pollution permits on an electricity
(and, where appropriate, thermal) output rather than on a
heat input basis, to encourage effi ciency in the use of fuel.
This Report
As indicated, this report addresses a broad range of source
categories. These sources do not represent the entire
inventory of PM
2.5
, SO
2
and NO
x
emissions, although they
do cover a large share ofthe national inventory. Each
source category chapter provides an overview ofthe
category, background on the technical as opposed to the
policy options for reducing emissions, and an overview of
existing regulatory authority (with the regulatory authority
issues discussed up-front in the mobile source chapters
because ofthe preeminence of preemption considerations).
Each chapter concludes with a discussion of state and local
policy measures.
Additionally, the report has two separate technology
chapters—one on boiler and another on diesel engine
technologies. The boiler technology chapter informs the
industrial and commercial boiler and electric generating
unit chapters, as well as the chapters on other source
categories that burn process fuels (e.g., pulp and paper).
The chapter on diesel engine technologies is useful for
understanding the three mobile source chapters, as well
as substantial portions ofthe airport and marine port
chapters.
The report begins with theThe Highlights ofthe source
category chapters. Although these do not substitute for
the detail provided in each chapter, they cull the most
signifi cant emissions reductions opportunities. Prior
to the sector-specifi c chapters, Chapter 2 discusses the
health effects of PM
2.5
, Chapter 3 discusses the national
emissions inventory, and Chapter 4 provides an overview
of theCleanAir Act.
References
Elliott, R. Neal, and M. Spurr, American Council for an
Energy-Effi cient Economy. Combined Heat and Power:
4 ControllingFineParticulateMatterUndertheCleanAirAct:AMenuof Options
Capturing Wasted Energy, May 1999. http://www.aceee.
org/pubs/IE983.htm.
U.S. Environmental Protection Agency (EPA). Combined
Heat and Power, January 2000. http://yosemite.epa.gov/
oar/globalwarming.nsf/UniqueKeyLookup/SHSU5BPLD4/
$File/combinedheatandpower.pdf.
State and Territorial Air Pollution Program Administrators
and the Association of Local Air Pollution Control Offi cials
(STAPPA/ALAPCO). Restrictions on the Stringency
of State and Local Air Quality Programs: Results ofa
Survey by the State and Territorial Air Pollution Program
Administrators (STAPPA) and the Association of Local
Air Pollution Control Offi cials (ALAPCO), December 17,
2002. http://www.4cleanair.org/stringency-report.pdf.
[...]... National Ambient Air Quality Standards for ParticulateMatter (Second Draft PM Staff Paper, January 2005): A Review by theParticulateMatter Review Panel ofthe EPA CleanAir Scientific Advisory Committee (EPASAB-CASAC-05-007), June 2005 www.epa.gov/sab /pdf/ casac-05-007 .pdf (2005b) Chapter 2 - Effects ofParticulateMatter on Human Health and the Environment 21 Chapter 3 FineParticulateMatter and... recently there has been a comprehensive reanalysis of data from the Six Cities and ACS studies, and new analyses using updated data from the AHSMOG and ACS ControllingFineParticulateMatterUndertheCleanAirAct:AMenuofOptions studies The reanalysis ofthe Six Cities and ACS studies confirms their original findings, suggesting an association with both total and cardiorespiratory mortality and exposure... national and regional approaches to achieving more stringent and expeditious reductions than CAIR STAPPA and ALAPCO’s strategy calls for a national SO2 cap of 1.26–1.89 million tons per year (as compared to a baseline of 10.6 million tons in 2001) by 2013, and a NOx cap of 0.88–1.26 million tons ControllingFineParticulateMatterUndertheCleanAirAct:AMenuofOptions per year by the same date (as compared... Luepker, M Mittleman, J Samet, S.C Smith, Jr, and I Tager Air Pollution and Cardiovascular Disease: A Statement for Healthcare Professionals from the Expert Panel on Population and Prevention Science of the American Heart Association,” Circulation 109: ControllingFineParticulateMatterUndertheCleanAirAct:AMenuofOptions 2655-71, June 1, 2004 reprint/109/21/2655 .pdf http://circ.ahajournals.org/cgi/... to date, however, areas throughout the eastern U.S and California exceed EPA’s National Ambient Air Quality Standards (NAAQS) for PM2.5 In this chapter, we discuss the characteristics of ambient PM, including size and chemical composition We also discuss the sources that contribute to ambient PM2.5 concentrations 22 ControllingFineParticulateMatterUndertheCleanAirAct:AMenuofOptions diameter,... effects of PM on materials have been investigated for metals, wood, stone, painted surfaces, electronics and fabrics Particulate pollution may soil and discolor these materials, reducing their aesthetic appeal It may also cause other physical and chemical degradation of materials through the action of acidic particles PM NAAQS Review As discussed in Chapter 3, EPA is required by the Clean Air Act to... for the irregular shape and varying density of most particles ControllingFineParticulateMatterUndertheCleanAirAct:AMenuofOptions distances by wind and weather, traveling thousands of miles from where they were formed Fig 2.1 The Human Respiratory System As discussed later in this report, the concentration and composition of particle pollution in the atmosphere vary by time of year and by... Phoenix PM2.5 Aerosol with the Unmix Receptor Model,” Journal of the Air and Waste Management Association, 53(3): 325-38, March 2003 Ramadan, Z., X.H Song, and P.K Hopke “Identification of Sources of Phoenix Aerosol by Positive Matrix Factorization,” Journal of the Air and Waste Management Association 50: 1308-1320, 2000 Sardar, S.B., P.M Fine, and C Sioutas “Seasonal and Spatial Variability ofthe Size-Resolved... http://cfpub.epa.gov/ncea/cfm/ partmatt.cfm (2004b) U.S Environmental Protection Agency (EPA) Review ofthe National Ambient Air Quality Standards for Particulate Matter: Policy Assessment of Scientific and Technical Information, OAQPS Staff Paper (EPA-452/R05-005), June 2005 www.epa.gov/ttnnaaqs/standards/pm/ data/pmstaffpaper_20050630 .pdf (200 5a) U.S Environmental Protection Agency (EPA) EPA’s Review ofthe National... Another major multi-city study used data from ten ofthe NMAPS cities where daily PM10 monitoring data were available (Schwartz, 2003) Again, the authors reported 18 a statistically significant association between PM10 and total mortality, with a reported health risk larger than that reported in the NMMAPS study The authors ofthe study suggest that the availability of more frequent monitoring data may partly . Particulate Matter
Under the Clean Air Act:
A Menu of Options
STAPPA
State and Territorial Air Pollution
Program Administrators
ALAPCO
Association of. Program
Administrators (STAPPA) and the Association of Local
Air Pollution Control Of cials (ALAPCO) are the two
national associations of air quality of